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If you go on a murdering spree and kill enough scientists (the Institute doesn’t seem to care too much if you destroy Synths) you’ll trigger the quest. You may want to wait until you get pulled into a meeting with several of them in the same room, which happens a few times. Emotionally it’s an easier route to take, but practically it's difficult, as you won't be right by the elevator. Kill two or three of these guys (Ayo, Holdren, Li, and / or Filmore) and the Institute won’t be happy. This is by far the easiest way to trigger Banished from the Institute, as he’s standing right by the elevator you need to use to escape. If you decide to kill Father ( brutal) you will instantly be branded a traitor, and on your way out someone will yell at you through a loudspeaker to make you feel bad.